TITLE

Vibration and two-photon absorption

AUTHOR(S)
Bishop, David M.; Luis, Josep M.; Kirtman, Bernard
PUB. DATE
June 2002
SOURCE
Journal of Chemical Physics;6/8/2002, Vol. 116 Issue 22, p9729
SOURCE TYPE
Academic Journal
DOC. TYPE
Article
ABSTRACT
A treatment of nuclear vibrational motions in two-photon absorption is laid out in detail. Perturbation theory is used to develop working formulas for diatomic molecules and tested for the X[sup 1]&sigma[sup +]-A[sup 1]Ï€ transition of carbon monoxide. The results are compared with the exact numerical values. Certain vibrational contributions, not previously recognized, are found to make an important contribution to the two-photon absorption probability.
ACCESSION #
6702796

 

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