First-, third-, and fifth-order resonant spectroscopy of an anharmonic displaced oscillators

Tanimura, Yoshitaka; Okumura, Ko
February 1997
Journal of Chemical Physics;2/8/1997, Vol. 106 Issue 6, p2078
Academic Journal
Discusses the Nth-order response functions for a two-level system described by displaced anharmonic potential surfaces coupled to a heat bath. Assumption that the heat-bath is an ensemble of harmonic oscillators; Bilinearity of coupling between the two-level system and the bath; Definition of the response functions in terms of line-shape functions.


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